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Lewis-acid Trapping of an Elusive Copper-Tosylnitrene Intermediate Using Scandium Triflate
High–valent copper nitrene intermediates have long been proposed to play a role in copper catalyzed aziridination and amination reactions. However, such intermediates have eluded detection for decades, which prevents the unambiguous assignments of mechanisms. Moreover, the electronic structure of th...
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| Main Authors: | , , , , , , , , |
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| Format: | Artigo |
| Jezik: | Inglês |
| Izdano: |
2012
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| Teme: | |
| Online dostop: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3743661/ https://ncbi.nlm.nih.gov/pubmed/22928636 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja306674h |
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