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Mechanistic and Computational Studies of Exocyclic Stereocontrol in the Synthesis of Bryostatin-like cis-2,6-Disubstituted-4-Alkylidene Tetrahydropyrans by Prins Cyclization
The Prins cyclization of syn-β-hydroxy allylsilanes and aldehydes gives cis-2,6-disubstituted 4-alkylidene tetrahydropyrans as sole products in excellent yields regardless of the aldehyde (R”) or syn-β-hydroxy allylsilane substituent (R’) used. By reversing the R” and R’ groups, complementary exocyc...
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| Main Authors: | , , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2012
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3537866/ https://ncbi.nlm.nih.gov/pubmed/23121542 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo301953h |
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