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Total Syntheses of Bryostatins. Syntheses of Two Ring-Expanded Bryostatin Analogues and Development of a New-Generation Strategy to Access the C7-C27 Fragment

This paper reports the synthesis of novel ring-expanded bryostatin analogues. By carefully modifying the substrate, a selective and high-yielding Ru-catalyzed tandem enyne coupling/Michael addition was employed to construct the northern fragment. A ring-closing metathesis was utilized to form the 31...

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Detalhes bibliográficos
Main Authors: Trost, Barry M., Yang, Hanbiao, Dong, Guangbin
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3517064/
https://ncbi.nlm.nih.gov/pubmed/21780195
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/chem.201002932
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