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Mechanistic Analysis of Gold(I)-Catalyzed Intramolecular Allene Hydroalkoxylation Reveals an Off-Cycle Bis(gold) Vinyl Species and Reversible C–O Bond Formation

Mechanistic investigation of gold(I)-catalyzed intramolecular allene hydroalkoxylation established a mechanism involving rapid and reversible C–O bond formation followed by turnover-limiting protodeauration from a mono(gold) vinyl complex. This on-cycle pathway competes with catalyst aggregation and...

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Main Authors: Brown, Timothy J., Weber, Dieter, Gagné, Michel R., Widenhoefer, Ross A.
Format: Artigo
Jezik:Inglês
Izdano: 2012
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC3433713/
https://ncbi.nlm.nih.gov/pubmed/22621418
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja303844h
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