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Active-Site Models for the Nickel-Iron Hydrogenases: Effects of Ligands on Reactivity and Catalytic Properties

Described are new derivatives of the type [HNiFe(SR)(2)(diphosphine)(CO)(3)](+), which feature a Ni(diphosphine) group linked to a Fe(CO)(3) group via two bridging thiolate ligands. Previous work had described [HNiFe(pdt)(dppe)(CO)(3)](+) ([1H](+)) and its activity as a catalyst for the reduction of...

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Detalhes bibliográficos
Main Authors: Carroll, Maria E., Barton, Bryan E., Gray, Danielle L., Mack, Amanda E., Rauchfuss, Thomas B.
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3183104/
https://ncbi.nlm.nih.gov/pubmed/21866886
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic2012759
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