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Efficient, scalable asymmetric synthesis of an epoxy quinol via Noyori desymmetrization of a meso diketone

Epoxy quinol 1a was prepared on a multi-gram scale by Noyori transfer hydrogenative desymmetrization of the readily available meso epoxy diketone 4. Although the intrinsic enantioselectivity for the desymmetrization was modest (82:18 er at 4% conversion), a highly enantiopure product (99.6:0.4 er) c...

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Detalhes bibliográficos
Main Authors: Clay, David R., Rosenberg, Ashley G., McIntosh, Matthias C.
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3131412/
https://ncbi.nlm.nih.gov/pubmed/21743778
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tetasy.2011.04.022
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