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Investigating Inner Sphere Reorganization via Secondary Kinetic Isotope Effects in the C–H Cleavage Reaction Catalyzed by Soybean Lipoxygenase: Tunneling in the Substrate Backbone as well as the Transferred Hydrogen

This work describes the application of NMR to the measurement of secondary deuterium (2° (2)H) and carbon-13 ((13)C) kinetic isotope effects (KIES) at positions 9 to 13 within the substrate linoleic acid (LA) of soybean lipoxygenase-1. The KIEs have been measured using linoleic acid labeled with eit...

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Detalhes bibliográficos
Main Authors: Meyer, Matthew P., Klinman, Judith P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3090704/
https://ncbi.nlm.nih.gov/pubmed/21192631
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja1050742
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