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Oxidative group transfer to a triiron complex to form a nucleophilic μ(3)-nitride, [Fe(3)(μ(3)-N)](−)

Utilizing a hexadentate ligand platform, a high-spin trinuclear iron complex of the type ((tbs)L)Fe(3)(thf) was synthesized and characterized ([(tbs)L](6−) = [1,3,5-C(6)H(9)(NPh-o-NSi(t)BuMe(2))(3)](6−)). The silyl-amide groups only permit ligation of one solvent molecule to the tri-iron core, resul...

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Autors principals: Powers, Tamara M., Fout, Alison R., Zheng, Shao-Liang, Betley, Theodore A.
Format: Artigo
Idioma:Inglês
Publicat: 2011
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC3056537/
https://ncbi.nlm.nih.gov/pubmed/21332160
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja2003445
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