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Testing the polynuclear hypothesis: multi-electron reduction of small molecules by triiron reaction sites
High-spin trinuclear iron complex ((tbs)L)Fe(3)(thf) ([(tbs)L](6−) = [1,3,5- C(6)H(9)(NPh-o-NSi(t)BuMe(2))(3)](6−)) (S = 6) facilitates 2 and 4e(−) reduction of N(x)H(y) type substrates to yield imido and nitrido products. Reaction of hydrazine or phenylhydrazine with ((tbs)L)Fe(3)(thf) yields triir...
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| Main Authors: | , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2013
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3801182/ https://ncbi.nlm.nih.gov/pubmed/23865953 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja405057n |
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