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Asymmetric Synthesis of All the Known Phlegmarine Alkaloids

The asymmetric synthesis of all four of the known natural phlegmarines and one synthetic derivative has been accomplished in 19 to 22 steps from 4-methoxy-3-(triisopropylsilyl)pyridine. Chiral N-acylpyridinium salt chemistry was used twice to set the stereocenters at the C-9 and C-2′ positions of th...

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Détails bibliographiques
Auteurs principaux: Wolfe, Bradley H., Libby, Adam H., Al-awar, Rima S., Foti, Christopher J., Comins, Daniel L.
Format: Artigo
Langue:Inglês
Publié: 2010
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC3006060/
https://ncbi.nlm.nih.gov/pubmed/21077636
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo1019688
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