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Synthesis of Enantioenriched α,α-Disubstituted Cyclopentenes Catalyzed by N-Heterocyclic Carbenes

The desymmetrization of 1,3-diketones using N-heterocyclic carbenes results in the formation of highly enantioenriched cyclopentenes in good yield. The reaction proceeds through a catalytic intramolecular aldol reaction and subsequent β-lactone formation. The expulsion of carbon dioxide at mild reac...

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Detalhes bibliográficos
Main Authors: Phillips, Eric M., Wadamoto, Manabu, Scheidt, Karl A.
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2981176/
https://ncbi.nlm.nih.gov/pubmed/21085623
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1055/s-0028-1083284
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