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Nonlinear optical spectroscopy of single, few, and many molecules; nonequilibrium Green’s function QED approach

Nonlinear optical signals from an assembly of N noninteracting particles consist of an incoherent and a coherent component, whose magnitudes scale ~ N and ~ N(N − 1), respectively. A unified microscopic description of both types of signals is developed using a quantum electrodynamical (QED) treatmen...

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Main Authors: Marx, Christoph A., Harbola, Upendra, Mukamel, Shaul
格式: Artigo
語言:Inglês
出版: 2008
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC2964889/
https://ncbi.nlm.nih.gov/pubmed/21037933
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1103/PhysRevA.77.022110
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