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Probing Electron Correlations in Molecules by Two-Dimensional Coherent Optical Spectroscopy
The nonlinear optical signal generated in phenol by three femtosecond pulses with wavevectors k(1), k(2), and k(3) in the phase-matching direction k(1) + k(2) − k(3) is simulated. This two-dimensional coherent spectroscopy (2DCS) signal has a rich pattern containing information on double-excitation...
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| Main Authors: | , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2008
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2901111/ https://ncbi.nlm.nih.gov/pubmed/18288841 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja0774414 |
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