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Probing Electron Correlations in Molecules by Two-Dimensional Coherent Optical Spectroscopy

The nonlinear optical signal generated in phenol by three femtosecond pulses with wavevectors k(1), k(2), and k(3) in the phase-matching direction k(1) + k(2) − k(3) is simulated. This two-dimensional coherent spectroscopy (2DCS) signal has a rich pattern containing information on double-excitation...

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Bibliographic Details
Main Authors: Li, Zhenyu, Abramavicius, Darius, Mukamel, Shaul
Format: Artigo
Language:Inglês
Published: 2008
Subjects:
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC2901111/
https://ncbi.nlm.nih.gov/pubmed/18288841
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja0774414
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