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Nonlinear optical spectroscopy of single, few, and many molecules; nonequilibrium Green’s function QED approach
Nonlinear optical signals from an assembly of N noninteracting particles consist of an incoherent and a coherent component, whose magnitudes scale ~ N and ~ N(N − 1), respectively. A unified microscopic description of both types of signals is developed using a quantum electrodynamical (QED) treatmen...
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| Main Authors: | , , |
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| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2008
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2964889/ https://ncbi.nlm.nih.gov/pubmed/21037933 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1103/PhysRevA.77.022110 |
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