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Mechanism of the Enantioselective Oxidation of Racemic Secondary Alcohols Catalyzed by Chiral Mn(III)–Salen Complexes

The experiments described here clarify the mechanism and origin of the enantioselectivity of the oxidation of racemic secondary alcohols catalyzed by chiral Mn(III)–salen complexes using HOBr, Br(2)/H(2)O/KOAc or PhI(OAc)(2)/H(2)O/KBr as a stoichiometric oxidant. Key points of the proposed pathway i...

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Detaylı Bibliyografya
Asıl Yazarlar: Brown, M. Kevin, Blewett, Megan M., Colombe, James R., Corey, E. J.
Materyal Türü: Artigo
Dil:Inglês
Baskı/Yayın Bilgisi: 2010
Konular:
Online Erişim:https://ncbi.nlm.nih.gov/pmc/articles/PMC2945693/
https://ncbi.nlm.nih.gov/pubmed/20666410
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja103103d
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