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Total Synthesis of (+)-Sieboldine A

The first total synthesis of (+)-sieboldine A was completed in 20 steps from readily available (3aS,6aR)-3,3a,4,6-atetrahydro-2H-cyclopenta[b]furan-2-one (5). Key steps are: (a) a pinacol-terminated 1,6-enyne cyclization reaction to form the cis-hydrindanone core (11 → 12), (b) formation of the spir...

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Autors principals: Canham, Stephen M., France, David J., Overman, Larry E.
Format: Artigo
Idioma:Inglês
Publicat: 2010
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2885033/
https://ncbi.nlm.nih.gov/pubmed/20527933
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja103666n
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