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Nature of Intermediates in Organo-SOMO Catalysis of α-Arylation of Aldehydes

The intramolecular α-arylation of aldehydes via organo-SOMO catalysis was investigated using density functional theory (B3LYP and M06-2X functionals). The geometries, spin densities, Mulliken charges, and molecular orbitals of the reacting enamine radical cations were analyzed, and the nature of the...

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Detalhes bibliográficos
Main Authors: Um, Joann M., Gutierrez, Osvaldo, Schoenebeck, Franziska, Houk, K. N., MacMillan, David W. C.
Formato: Artigo
Idioma:Inglês
Publicado em: 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2862978/
https://ncbi.nlm.nih.gov/pubmed/20387888
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9063074
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