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Asymmetric Synthesis, Structure, and Reactivity of Unexpectedly Stable Spiroepoxy-β-Lactones Including Facile Conversion to Tetronic Acids: Application to (+)-Maculalactone A

A novel class of small spirocyclic heterocycles, spiroepoxy-β-lactones (1,4-dioxaspiro[2.3]-hexan-5-ones), is described that exhibit a number of interesting reactivity patterns. These spiroheterocycles, including an optically active series, are readily synthesized by epoxidation of ketene dimers (4-...

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Detalhes bibliográficos
Main Authors: Duffy, Richard J., Morris, Kay A., Vallakati, Ravikrishna, Zhang, Wei, Romo, Daniel
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2745962/
https://ncbi.nlm.nih.gov/pubmed/19453152
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo900499e
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