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Substituent Effects on the Rearrangements of Cyclohexyl to Cyclopentyl Radicals Involving Avermectin-related Radicals

The rearrangement of a substituted cyclohexyl radical to a cyclopentylmethyl radical on the skeleton of Avermectin B(1) has been investigated using density functional (UB3LYP/6-31G(d)) and G3MP2B3 computational methods. The rearrangement is preferred when highly radical stabilizing groups are presen...

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Hlavní autoři: Luft, Jennifer A. R., Winkler, Tammo, Kessabi, Fiona M., Houk, K. N.
Médium: Artigo
Jazyk:Inglês
Vydáno: 2008
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC2652414/
https://ncbi.nlm.nih.gov/pubmed/18842059
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo800923a
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