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Effects of Thioether Substituents on the O(2) Reactivity of β-Diketiminate-Cu(I) Complexes: Probing the Role of the Methionine Ligand in Copper Monooxygenases

The activation of dioxygen by dopamine β-monooxygenase (DβM) and peptidylglycine α-hydroxylating monooxygenase (PHM) is postulated to occur at a copper site ligated by two histidine imidazoles and a methionine thioether, which is unusual since such thioether ligation is not present in other O(2)-act...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Hauptverfasser: Aboelella, Nermeen W., Gherman, Benjamin F., Hill, Lyndal M. R., York, John T., Holm, Nicole, Young, Victor G., Cramer, Christopher J., Tolman, William B.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2006
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2593856/
https://ncbi.nlm.nih.gov/pubmed/16522125
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja057745v
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