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A new paradigm for electrostatic catalysis of radical reactions in vitamin B(12) enzymes

The catalytic power of enzymes containing coenzyme B(12) cofactor has been, in some respects, the “last bastion” for the strain hypothesis. The present work explores the origin of this effect by using simulation methods that overcome the sampling difficulties of previous energy minimization studies....

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Detalhes bibliográficos
Main Authors: Sharma, Pankaz K., Chu, Zhen T., Olsson, Mats H. M., Warshel, Arieh
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC1887576/
https://ncbi.nlm.nih.gov/pubmed/17517615
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0702238104
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