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Stereoselective tandem iridium-catalyzed alkene isomerization-cope rearrangement of ω-diene epoxides: efficient access to acyclic 1,6-dicarbonyl compounds

The Cope rearrangement of 2,3-divinyloxiranes, a rare example of epoxide C–C bond cleavage, results in 4,5-dihydrooxepines which are amenable to hydrolysis, furnishing 1,6-dicarbonyl compounds containing two contiguous stereocenters at the 3- and 4-positions. We employ an Ir-based alkene isomerizati...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Suresh, Rahul, Massad, Itai, Marek, Ilan
Formato: Artigo
Idioma:Inglês
Publicado em: The Royal Society of Chemistry 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8278922/
https://ncbi.nlm.nih.gov/pubmed/34349902
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d1sc02575a
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