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How metallylenes activate small molecules

We have studied the activation of dihydrogen by metallylenes using relativistic density functional theory (DFT). Our detailed activation strain and Kohn–Sham molecular orbital analyses have quantified the physical factors behind the decreased reactivity of the metallylene on going down Group 14, fro...

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書目詳細資料
發表在:Chem Sci
Main Authors: Vermeeren, Pascal, Doppert, Michael T., Bickelhaupt, F. Matthias, Hamlin, Trevor A.
格式: Artigo
語言:Inglês
出版: The Royal Society of Chemistry 2021
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC8179460/
https://ncbi.nlm.nih.gov/pubmed/34163718
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0sc05987k
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