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Sulfamides direct radical-mediated chlorination of aliphatic C–H bonds

Given the prevalence of aliphatic amines in bioactive small molecules, amine derivatives are opportune as directing groups. Herein, sulfamides serve as amine surrogates to guide intermolecular chlorine-transfer at γ-C(sp(3)) centers. This unusual position-selectivity arises because accessed sulfamid...

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Détails bibliographiques
Publié dans:Chem Sci
Auteurs principaux: Short, Melanie A., Shehata, Mina F., Sanders, Matthew A., Roizen, Jennifer L.
Format: Artigo
Langue:Inglês
Publié: The Royal Society of Chemistry 2019
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC8132995/
https://ncbi.nlm.nih.gov/pubmed/34040715
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc03428e
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