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Sulfamyl Radicals Direct Photoredox-Mediated Giese Reactions at Unactivated C(3)–H Bonds

Alcohol-anchored sulfamate esters guide the alkylation of tertiary and secondary aliphatic C(3)–H bonds. The transformation proceeds directly from N–H bonds with a catalytic oxidant, a contrast to prior methods which have required pre-oxidation of the reactive nitrogen center, or employed stoichiome...

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Détails bibliographiques
Publié dans:Org Lett
Auteurs principaux: Kanegusuku, Anastasia L. G., Castanheiro, Thomas, Ayer, Suraj K., Roizen, Jennifer L.
Format: Artigo
Langue:Inglês
Publié: 2019
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC7359209/
https://ncbi.nlm.nih.gov/pubmed/31313933
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.9b02234
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