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Biosynthesis of the Immunosuppressant (−)-FR901483
We report characterization of the biosynthetic pathway of the potent immunosuppressant (−)-FR901483 (1) through heterologous expression and enzymatic assays. The biosynthetic logic to form the azatricyclic alkaloid is consistent with those proposed in biomimetic syntheses, and involves aza-spiro ann...
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| Publicado no: | J Am Chem Soc |
|---|---|
| Main Authors: | , , , , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2020
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC8094545/ https://ncbi.nlm.nih.gov/pubmed/33372776 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c12352 |
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