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S-Adenosyl-l-ethionine is a Catalytically Competent Analog of S-Adenosyl-l-methione (SAM) in the Radical SAM Enzyme HydG
Radical S-adenosyl-l-methionine (SAM) enzymes initiate biological radical reactions with the 5’-deoxyadenosyl radical (5’-dAdo•). A [4Fe-4S](+) cluster reductively cleaves SAM to form the Ω organometallic intermediate in which the 5’-deoxyadenosyl moiety is directly bound to the unique iron of the [...
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| Publicado no: | Angew Chem Int Ed Engl |
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| Main Authors: | , , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2020
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC8081114/ https://ncbi.nlm.nih.gov/pubmed/33935588 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202014337 |
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