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Closed Shell Iron(IV) Oxo Complex with an Fe–O Triple Bond: Computational Design, Synthesis, and Reactivity

Iron(IV)‐oxo intermediates in nature contain two unpaired electrons in the Fe–O antibonding orbitals, which are thought to contribute to their high reactivity. To challenge this hypothesis, we designed and synthesized closed‐shell singlet iron(IV) oxo complex [(quinisox)Fe(O)](+) (1(+); quinisox‐H=(...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Andris, Erik, Segers, Koen, Mehara, Jaya, Rulíšek, Lubomír, Roithová, Jana
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7756500/
https://ncbi.nlm.nih.gov/pubmed/32926539
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202009347
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