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Unexpected enzyme-catalysed [4+2] cycloaddition and rearrangement in polyether antibiotic biosynthesis

Enzymes catalysing remarkable Diels-Alder-like [4+2] cyclisations have been previously implicated in the biosynthesis of spirotetronate and spirotetramate antibiotics. Biosynthesis of the polyether antibiotic tetronasin is not anticipated to require such steps, yet the tetronasin gene cluster encode...

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Detalhes bibliográficos
Publicado no:Nat Catal
Main Authors: Little, Rory, Paiva, Fernanda C. R., Jenkins, Rob, Hong, Hui, Sun, Yuhui, Demydchuk, Yuliya, Samborskyy, Markiyan, Tosin, Manuela, Leeper, Finian J., Dias, Marcio V. B., Leadlay, Peter F.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7617221/
https://ncbi.nlm.nih.gov/pubmed/39659772
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41929-019-0351-2
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