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Highly Diastereoselective Functionalization of Piperidines by Photoredox Catalyzed α-Amino C–H Arylation and Epimerization

We report a photoredox catalyzed α-amino C–H arylation reaction of highly substituted piperidine derivatives with electron deficient cyano(hetero)arenes. The scope and limitations of the reaction were explored, with piperidines bearing multiple substitution patterns providing the arylated products i...

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Detalles Bibliográficos
Publicado en:J Am Chem Soc
Main Authors: Walker, Morgan M., Koronkiewicz, Brian, Chen, Shuming, Houk, K. N., Mayer, James M., Ellman, Jonathan A.
Formato: Artigo
Idioma:Inglês
Publicado: 2020
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC7318553/
https://ncbi.nlm.nih.gov/pubmed/32286827
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b13165
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