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Performance of Localized Coupled Cluster Methods in a Moderately Strong Correlation Regime: Hückel–Möbius Interconversions in Expanded Porphyrins

[Image: see text] Localized orbital coupled cluster theory has recently emerged as a nonempirical alternative to DFT for large systems. Intuitively, one might expect such methods to perform less well for highly delocalized systems. In the present work, we apply both canonical CCSD(T) approximations...

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Publicat a:J Chem Theory Comput
Autors principals: Sylvetsky, Nitai, Banerjee, Ambar, Alonso, Mercedes, Martin, Jan M. L.
Format: Artigo
Idioma:Inglês
Publicat: American Chemical Society 2020
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC7304861/
https://ncbi.nlm.nih.gov/pubmed/32338891
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jctc.0c00297
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