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Performance of Localized Coupled Cluster Methods in a Moderately Strong Correlation Regime: Hückel–Möbius Interconversions in Expanded Porphyrins

[Image: see text] Localized orbital coupled cluster theory has recently emerged as a nonempirical alternative to DFT for large systems. Intuitively, one might expect such methods to perform less well for highly delocalized systems. In the present work, we apply both canonical CCSD(T) approximations...

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Pubblicato in:J Chem Theory Comput
Autori principali: Sylvetsky, Nitai, Banerjee, Ambar, Alonso, Mercedes, Martin, Jan M. L.
Natura: Artigo
Lingua:Inglês
Pubblicazione: American Chemical Society 2020
Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC7304861/
https://ncbi.nlm.nih.gov/pubmed/32338891
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jctc.0c00297
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