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Reduction of a dihydroboryl cation to a boryl anion and its air-stable, neutral hydroboryl radical through hydrogen shuttling

The addition of Lewis bases to a cyclic (alkyl)(amino)carbene (CAAC)-supported dihydroboron triflate yields the mixed doubly base-stabilised dihydroboryl cations [(CAAC)BH(2)L](+). Of these, [(CAAC)(2)BH(2)]OTf (OTf = triflate) underwent facile two-electron reduction with KC(8) owing to a 1,2-hydrid...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Hagspiel, Stephan, Arrowsmith, Merle, Fantuzzi, Felipe, Hermann, Alexander, Paprocki, Valerie, Drescher, Regina, Krummenacher, Ivo, Braunschweig, Holger
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7069503/
https://ncbi.nlm.nih.gov/pubmed/32206272
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc05026d
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