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Synthesis of Chiral Tetrasubstituted Azetidines from Donor–Acceptor Azetines via Asymmetric Copper(I)-Catalyzed Imido-Ylide [3+1]-Cycloaddition with Metallo-Enolcarbenes

The all-cis stereoisomers of tetrasubstituted azetidine-2-carboxylic acids and derivatives that possess three chiral centers have been prepared in high yield and stereocontrol from silyl-protected Z-γ-substituted enoldiazoacetates and imido-sulfur ylides by asymmetric [3+1]-cycloaddition using chira...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Marichev, Kostiantyn O., Wang, Kan, Dong, Kuiyong, Greco, Nicole, Massey, Lynée A., Deng, Yongming, Arman, Hadi, Doyle, Michael P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7027963/
https://ncbi.nlm.nih.gov/pubmed/31496021
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201909929
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