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Triarylaminium Radical Cation Promoted Coupling of Catharanthine with Vindoline: Diastereospecific Synthesis of Anhydrovinblastine and Reaction Scope

A new triarylaminium radical cation promoted coupling of catharanthine with vindoline is disclosed, enlisting tris(4-bromophenyl)aminium hexachlororantimonate (BAHA, 1.1 equiv) in aqueous 0.05 N HCl/trifluoroethanol (1–10:1) at room temperature (25 °C), that provides anhydrovinblastine in superb yie...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Boon, Byron A., Boger, Dale L.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6750708/
https://ncbi.nlm.nih.gov/pubmed/31442047
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b06968
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