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Total Synthesis of (–)-Salinosporamide A via a Late Stage C-H Insertion

The synthesis of (–)-salinosporamide A, a proteasome inhibitor, is described. The synthesis highlights the assembly of a densely decorated pyrrolidinone core via an aza-Payne/hydroamination sequence. Central to the success of the synthesis is a late stage C–H insertion reaction to functionalize a st...

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Dades bibliogràfiques
Publicat a:Angew Chem Int Ed Engl
Autors principals: Gholami, Hadi, Kulshrestha, Aman, Favor, Olivia K., Staples, Richard J., Borhan, Babak
Format: Artigo
Idioma:Inglês
Publicat: 2019
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6715302/
https://ncbi.nlm.nih.gov/pubmed/30887693
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201900340
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