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Light Enhanced Fe-Mediated Nitrogen Fixation: Mechanistic Insights Regarding H(2) Elimination, HER, and NH(3) Generation
Despite their proposed accumulation at the Fe sites of the FeMo-cofactor of MoFe-nitrogenase, the presence of hydride ligands in molecular model systems capable of the nitrogen reduction reaction (N(2)RR) appears to diminish the catalytic N(2)-to-NH(3) conversion. We find that for an iron-based syst...
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| Publicado no: | ACS Catal |
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| Main Authors: | , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2019
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6715299/ https://ncbi.nlm.nih.gov/pubmed/31467770 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acscatal.9b00523 |
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