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Regiodivergent Photocyclization of Dearomatized Acylphloroglu-cinols: Asymmetric Syntheses of (−)-Nemorosone and (−)-6-epi-Garcimultiflorone A

Regiodivergent photocyclization of dearomatized acylphloroglucinol substrates has been developed to produce type A polycyclic polyprenylated acylphloroglucinol (PPAP) derivatives using an excited-state intramolecular proton transfer (ESIPT) process. Using this strategy, we achieved the enantioselect...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Wen, Saishuai, Boyce, Jonathan H., Kandappa, Sunil K., Sivaguru, Jayaraman, Porco, John A.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6659400/
https://ncbi.nlm.nih.gov/pubmed/31264859
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b05600
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