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Geometric and Electronic Structure Contributions to O–O Cleavage and the Resultant Intermediate Generated in Heme-Copper Oxidases
This study investigates the mechanism of O–O bond cleavage in heme-copper oxidase (HCO) enzymes, combining experimental and computational insights from enzyme intermediates and synthetic models. It is determined that HCOs undergo a proton-initiated O–O cleavage mechanism where a single water molecul...
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| Publicado no: | J Am Chem Soc |
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| Principais autores: | , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2019
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6639083/ https://ncbi.nlm.nih.gov/pubmed/31146528 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b04271 |
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