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Tandem Catalysis: Transforming Alcohols to Alkenes by Oxidative Dehydroxymethylation

We report a Rh-catalyst for accessing olefins from primary alcohols by a C–C bond cleavage that results in dehomologation. This functional group interconversion proceeds by an oxidation-dehydroformylation enabled by N,N-dimethylacrylamide as a sacrificial acceptor of hydrogen gas. Alcohols with dive...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Wu, Xuesong, Cruz, Faben A., Lu, Alexander, Dong, Vy M.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6619493/
https://ncbi.nlm.nih.gov/pubmed/30084247
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b06069
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