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Electronic Structures of an [Fe(NNR(2))](+/0/-) Redox Series: Ligand Noninnocence and Implications for Catalytic Nitrogen Fixation
The intermediacy of metal-NNH(2) complexes has been implicated in the catalytic cycles of several examples of transition-metal-mediated nitrogen (N(2)) fixation. In this context, we have shown that triphosphine-supported Fe(N(2)) complexes can be reduced and protonated at the distal N atom to yield...
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| Udgivet i: | Inorg Chem |
|---|---|
| Main Authors: | , , , , , , , , |
| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2019
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6598684/ https://ncbi.nlm.nih.gov/pubmed/30762355 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.inorgchem.9b00133 |
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