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Brønsted acid and Pd–PHOX dual-catalysed enantioselective addition of activated C-pronucleophiles to internal dienes

We describe the development of Pd–PHOX-catalysed enantioselective couplings of internal dienes with malononitrile and other activated C-pronucleophiles. Reactions are dramatically accelerated by the addition of Et(3)N·HBAr(F)(4) as a Brønsted acid co-catalyst, enabling a suite of products bearing a...

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Détails bibliographiques
Publié dans:Chem Sci
Auteurs principaux: Park, Sangjune, Adamson, Nathan J., Malcolmson, Steven J.
Format: Artigo
Langue:Inglês
Publié: Royal Society of Chemistry 2019
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC6524568/
https://ncbi.nlm.nih.gov/pubmed/31183071
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc00633h
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