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Hyperconjugative Aromaticity and Antiaromaticity Control the Reactivities and π-Facial Stereoselectivities of 5-Substituted Cyclopentadiene Diels–Alder Cycloadditions

The reactivities and π-facial stereoselectivities of Diels–Alder reactions of 5-substituted cyclopentadienes were studied using density functional theory. Burnell and co-workers previously showed that the π-facial selectivities result from the energies required to distort the reactants into the tran...

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Detalhes bibliográficos
Publicado no:J Org Chem
Main Authors: Levandowski, Brian J., Zou, Lufeng, Houk, K. N.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6467786/
https://ncbi.nlm.nih.gov/pubmed/30395708
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.joc.8b02537
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