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Hyperconjugative Antiaromaticity Activates 4H-Pyrazoles as Inverse-Electron Demand Diels–Alder Dienes
The Diels–Alder reactivity of 4,4-difluoro-3,5-diphenyl-4H-pyrazole (DFP) was investigated experimentally and computationally with endo-bicyclo[6.1.0]non-4-yne (BCN). The computationally predicted rate enhancement from hyperconjugative antiaromaticity induced by fluorination of cyclopentadienes at t...
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| Publicado no: | Org Lett |
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| Main Authors: | , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2019
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC7015664/ https://ncbi.nlm.nih.gov/pubmed/31589054 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.9b03351 |
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