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Arynes and Cyclic Alkynes as Synthetic Building Blocks for Stereodefined Quaternary Centers

We report a facile method to synthesize stereodefined quaternary centers from reactions of arynes and related strained intermediates using β-ketoester-derived substrates. The conversion of β- ketoesters to chiral enamines is followed by reaction with in situ generated strained arynes or cyclic alkyn...

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Veröffentlicht in:J Am Chem Soc
Hauptverfasser: Picazo, Elias, Anthony, Sarah M., Giroud, Maude, Simon, Adam, Miller, Margeaux A., Houk, K. N., Garg, Neil K.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2018
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6467087/
https://ncbi.nlm.nih.gov/pubmed/29716194
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b02875
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