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Characterized cis-Fe(V)(O)(OH) intermediate mimics enzymatic oxidations in the gas phase

Fe(V)(O)(OH) species have long been proposed to play a key role in a wide range of biomimetic and enzymatic oxidations, including as intermediates in arene dihydroxylation catalyzed by Rieske oxygenases. However, the inability to accumulate these intermediates in solution has thus far prevented thei...

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Detalhes bibliográficos
Publicado no:Nat Commun
Main Authors: Borrell, Margarida, Andris, Erik, Navrátil, Rafael, Roithová, Jana, Costas, Miquel
Formato: Artigo
Idioma:Inglês
Publicado em: Nature Publishing Group UK 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6385299/
https://ncbi.nlm.nih.gov/pubmed/30796210
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41467-019-08668-2
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