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Reversible homolytic activation of water via metal–ligand cooperativity in a T-shaped Ni(ii) complex

A T-shaped Ni(ii) complex [(Tol,Ph)DHPy]Ni has been prepared and characterized. EPR spectra and DFT calculations of this complex suggest that the electronic structure is best described as a high-spin Ni(ii) center antiferromagnetically coupled with a ligand-based radical. This complex reacts with wa...

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Vydáno v:Chem Sci
Hlavní autoři: Chang, Mu-Chieh, Jesse, Kate A., Filatov, Alexander S., Anderson, John S.
Médium: Artigo
Jazyk:Inglês
Vydáno: Royal Society of Chemistry 2018
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC6354739/
https://ncbi.nlm.nih.gov/pubmed/30809351
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c8sc03719a
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