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Biosynthesis of Heptacyclic Duclauxins Requires Extensive Redox Modifications of the Phenalenone Aromatic Polyketide

Duclauxins are dimeric and heptacyclic fungal polyketides significant bioactivities. We characterized the cascade of redox transformations in the biosynthesis of duclauxin pathway from Talaromyces stipitatus. The redox reaction sequence is initiated by a cupin family dioxygenase DuxM that performs a...

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Vydáno v:J Am Chem Soc
Hlavní autoři: Gao, Shu-Shan, Zhang, Tao, Garcia-Borràs, Marc, Hung, Yiu-Sun, Billingsley, John M, Houk, K. N., Hu, Youcai, Tang, Yi
Médium: Artigo
Jazyk:Inglês
Vydáno: 2018
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC6309916/
https://ncbi.nlm.nih.gov/pubmed/29741874
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b03705
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