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Total Synthesis of Unsymmetrically Oxidized Nuphar Thioalkaloids via Copper-Catalyzed Thiolane Assembly

An asymmetric total synthesis of (+)-6-hydroxythiobinupharidine (1b) and (−)-6-hydroxythionuphlutine (2b), a set of hemiaminal containing dimeric sesquiterpenes isolated from yellow water lilies of the Nuphar genus, is described. The central bis-spirocyclic tetrahydrothiophene ring was forged throug...

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Vydáno v:J Am Chem Soc
Hlavní autoři: Lacharity, Jacob J., Fournier, Jeremy, Lu, Ping, Mailyan, Artur K., Herrmann, Aaron T., Zakarian, Armen
Médium: Artigo
Jazyk:Inglês
Vydáno: 2017
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC6309176/
https://ncbi.nlm.nih.gov/pubmed/28911224
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b07685
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