Bulk-to-Surface Proton-Coupled Electron Transfer Reactivity of the Metal−Organic Framework MIL-125

Stoichiometric proton-coupled electron transfer (PCET) reactions of the metal−organic framework (MOF) MIL-125, Ti(8)O(8)(OH)(4)(bdc)(6) (bdc = terephthalate), are described. In the presence of UV light and 2-propanol, MIL-125 was photoreduced to a maximum of 2(e(−)/H(+)) per Ti(8) node. This stoichi...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Saouma, Caroline T., Richard, Sarah, Smolders, Simon, Delley, Murielle F., Ameloot, Rob, Vermoortele, Frederik, De Vos, Dirk E., Mayer, James M.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
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Article
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6276121/
https://ncbi.nlm.nih.gov/pubmed/30392350
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b09120
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